Recent Development in Tem Characterization of Irradiated Rertr Fuels

Recent Development in Tem Characterization of Irradiated Rertr Fuels

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Published: 2011

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The recent development on TEM work of irradiated RERTR fuels includes microstructural characterization of the irradiated U-10Mo/alloy-6061 monolithic fuel plate, the RERTR-7 U-7Mo/Al-2Si and U-7Mo/Al-5Si dispersion fuel plates. It is the first time that a TEM sample of an irradiated nuclear fuel was prepared using the focused-ion-beam (FIB) lift-out technical at the Idaho National Laboratory. Multiple FIB TEM samples were prepared from the areas of interest in a SEM sample. The characterization was carried out using a 200kV TEM with a LaB6 filament. The three dimensional orderings of nanometer-sized fission gas bubbles are observed in the crystalline region of the U-Mo fuel. The co-existence of bubble superlattice and dislocations is evident. Detailed microstructural information along with composition analysis is obtained. The results and their implication on the performance of these fuels are discussed.


Characterization of an Irradiated RERTR-7 Fuel Plate Using Transmission Electron Microscopy

Characterization of an Irradiated RERTR-7 Fuel Plate Using Transmission Electron Microscopy

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Published: 2010

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Transmission electron microscopy (TEM) has been used to characterize an irradiated fuel plate with Al-2Si matrix from the RERTR-7 experiment that was irradiated under moderate reactor conditions. The results of this work showed the presence of a bubble superlattice within the U-7Mo grains that accommodated fission gases (e.g., Xe). The presence of this structure helps the U-7Mo exhibit a stable swelling behaviour during irradiation. Furthermore, TEM analysis showed that the Si-rich interaction layers that develop around the fuel particles at the U-7Mo/matrix interface during fuel plate fabrication and irradiation become amorphous during irradiation, and in regions of the interaction layer that have relatively high Si concentrations the fission gas bubbles remain small and contained within the layer but in areas with lower Si concentrations the bubbles grow in size. An important question that remains to be answered about the irradiation behaviour of U-Mo dispersion fuels, is how do more aggressive irradiation conditions affect the behaviour of fission gases within the U-7Mo fuel particles and in the amorphous interaction layers on the microstructural scale that can be characterized using TEM? This paper discusses the results of TEM analysis that was performed on a sample taken from an irradiated RERTR-7 fuel plate with Al-2Si matrix. This plate was exposed to more aggressive irradiation conditions than was the sample taken from the RERTR-6 plate. The microstructural features present within the U-7Mo and the amorphous interaction layers will be discussed. The results of this analysis will be compared to what was observed in the earlier RERTR-6 fuel plate characterization.


Microstructure Characterization of RERTR Fuel

Microstructure Characterization of RERTR Fuel

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Published: 2008

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A variety of phases have the potential to develop in the irradiated fuels for the reduced enrichment research test reactor (RERTR) program. To study the radiation stability of these potential phases, three depleted uranium alloys were cast. The phases of interest were identified including U(Si, Al)3, (U, Mo)(Si, Al)3, UMo2Al20, UAl4, and U6Mo4Al43. These alloys were irradiated with 2.6 MeV protons at 200ðC up to 3.0 dpa. The microstructure is characterized using SEM and TEM. Microstructural characterization for an archive dispersion fuel plate (U-7Mo fuel particles in Al-2%Si cladding) was also carried out. TEM sample preparation for the irradiated dispersion fuel has been developed.


Tem Characterization of Irradiated U3SI2/AL Dispersion Fuel

Tem Characterization of Irradiated U3SI2/AL Dispersion Fuel

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Published: 2010

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The silicide dispersion fuel of U3Si2/Al has been recognized as a reasonably good performance fuel for nuclear research and test reactors except that it requires the use of high enrichment uranium. An irradiated U3Si2/Al dispersion fuel (~75% enrichment) from the high flux side of a RERTR-8 (U0R040) plate was characterized using transmission electron microscopy (TEM). The fuel plate was irradiated in the advanced test reactor (ATR) for 105 days. The average irradiation temperature and fission density of the fuel particles for the TEM sample are estimated to be approximately ~110 degrees C and 5.4 x 10-21 f/cm3. The characterization was performed using a 200KV TEM with a LaB6 filament. Detailed microstructural information along with composition analysis is obtained. The results and their implication on the performance of this silicide fuel are discussed.


Post-irradiation Examination Techniques for Research Reactor Fuels

Post-irradiation Examination Techniques for Research Reactor Fuels

Author: IAEA

Publisher: International Atomic Energy Agency

Published: 2023-04-18

Total Pages: 149

ISBN-13: 920102021X

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Post-irradiation examination (PIE) is an indispensable step in the selection of new or improved research reactor fuel, and in the characterization and understanding of its in-core behaviour. This publication provides an introduction to PIE techniques. It describes a typical PIE process from intercycle inspections in the reactor pool or channel, to hot cell PIE, which is subdivided into non-destructive and destructive testing techniques with their typical output, advantages and drawbacks, and their applicability to understanding fuel irradiation behaviour. Much of the work presented in this publication originated from the research and development of new low enriched uranium research reactor fuels. Intended readers include research reactor operators, regulators and their technical support organizations, fuel developers and manufacturers, laboratory staff, and policy makers.


RERTR Program Progress in Qualifying Reduced-enrichment Fuels

RERTR Program Progress in Qualifying Reduced-enrichment Fuels

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Published: 1982

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In order to provide the technical means for reducing the enrichment of uranium used to fuel research and test reactors, the US Reduced Enrichment Research and Test Reactor (RERTR) Program has been engaged in the development and testing of higher-uranium-density fuels than had been used previously. The main characteristics to be considered in evaluating the performance of a fuel are its swelling, its blister-threshold temperature, and its metallurgical appearance. Data for the qualification of the reduced-enrichment fuels being developed by the RERTR Program are obtained from examination of minature fuel plates (miniplates) which successfully pass the irradiation screening tests and from examinations of full-sized fuel elements. This paper will summarize the miniplate data and will give the status of full-sized element irradiations. Finally, the current status of qualification of the various fuel types will be discussed and some projections of the future will be given.


Stability Study of the RERTR Fuel Microstructure

Stability Study of the RERTR Fuel Microstructure

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Published: 2014

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The irradiation stability of the interaction phases at the interface of fuel and Al alloy matrix as well as the stability of the fission gas bubble superlattice is believed to be very important to the U-Mo fuel performance. In this paper the recent result from TEM characterization of Kr ion irradiated U-10Mo-5Zr alloy will be discussed. The focus will be on the phase stability of Mo2-Zr, a dominated second phase developed at the interface of U-10Mo and the Zr barrier in a monolithic fuel plate from fuel fabrication. The Kr ion irradiations were conducted at a temperature of 200 degrees C to an ion fluence of 2.0E+16 ions/cm2. To investigate the thermal stability of the fission gas bubble superlattice, a key microstructural feature in both irradiated dispersion U-7Mo fuel and monolithic U-10Mo fuel, a FIB-TEM sample of the irradiated U-10Mo fuel (3.53E+21 fission/cm3) was used for a TEM in-situ heating experiment. The preliminary result showed extraordinary thermal stability of the fission gas bubble superlattice. The implication of the TEM observation from these two experiments on the fuel microstructural evolution under irradiation will be discussed.


Irradiation Performance of Reduced-enrichment Fuels Tested Under the US RERTR Program

Irradiation Performance of Reduced-enrichment Fuels Tested Under the US RERTR Program

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Published: 1985

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Considerable progress in the irradiation testing of high-density, reduced-enrichment fuels has been made during the past year. Miniplates containing UA1, U3Si2, U3Si/sub 1.5/, U3Si, U3SiCu, and, U6Fe have been irradiated. Postirradiation examinations have revealed that breakway swelling has occurred in 6.4-Mg U/m3 U3Si plates at approx. 2.8 x 1027 fissions/m3. U3Si2 plates are continuing to show satisfactory performance. The testing of full-sized fuel elements in the ORR and the SILOE reactor have continued with good results. Postirradiation examinations are confirming the satisfactory performance of these elements.


US RERTR FUEL DEVELOPMENT POST IRRADIATION EXAMINATION RESULTS.

US RERTR FUEL DEVELOPMENT POST IRRADIATION EXAMINATION RESULTS.

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Published: 2008

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Post irradiation examinations of irradiated RERTR plate type fuel at the Idaho National Laboratory have led to in depth characterization of fuel behavior and performance. Both destructive and non-destructive examination capabilities at the Hot Fuels Examination Facility (HFEF) as well as recent results obtained are discussed herein. New equipment as well as more advanced techniques are also being developed to further advance the investigation into the performance of the high density U-Mo fuel.