Phononic and Electronic Excitations in Complex Oxides Studied with Advanced Infrared and Raman Spectroscopy Techniques

Phononic and Electronic Excitations in Complex Oxides Studied with Advanced Infrared and Raman Spectroscopy Techniques

Author: Fryderyk Lyzwa

Publisher: Springer Nature

Published: 2022-10-05

Total Pages: 158

ISBN-13: 3031118669

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This PhD thesis reports on investigations of several oxide-based materials using advanced infrared and Raman spectroscopy techniques and in combination with external stimuli such as high magnetic or electric field, sptial confinement in thin film heterostructures and the radiation with UV light. This leads to new results in the fields of superconductivity, electronic polarization states and nanoscale phenomena. Among these, the observation of anomalous polar moments is of great relevance for understanding the electric-field-induced metal-to-insulator transistion; and the demonstration that confocal Raman spectroscopy of backfolded acoustic photons in metal-oxide multilayers can be used as a powerful characterization tool for monitoring their interface properties and layer thickness is an important technical development for the engineering of such functional oxide heterostructures.


Synchrotron Light Sources and Free-Electron Lasers

Synchrotron Light Sources and Free-Electron Lasers

Author: Eberhard J. Jaeschke

Publisher: Springer

Published: 2016-05-27

Total Pages: 0

ISBN-13: 9783319143934

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Hardly any other discovery of the nineteenth century did have such an impact on science and technology as Wilhelm Conrad Röntgen’s seminal find of the X-rays. X-ray tubes soon made their way as excellent instruments for numerous applications in medicine, biology, materials science and testing, chemistry and public security. Developing new radiation sources with higher brilliance and much extended spectral range resulted in stunning developments like the electron synchrotron and electron storage ring and the freeelectron laser. This handbook highlights these developments in fifty chapters. The reader is given not only an inside view of exciting science areas but also of design concepts for the most advanced light sources. The theory of synchrotron radiation and of the freeelectron laser, design examples and the technology basis are presented. The handbook presents advanced concepts like seeding and harmonic generation, the booming field of Terahertz radiation sources and upcoming brilliant light sources driven by laser-plasma accelerators. The applications of the most advanced light sources and the advent of nanobeams and fully coherent x-rays allow experiments from which scientists in the past could not even dream. Examples are the diffraction with nanometer resolution, imaging with a full 3D reconstruction of the object from a diffraction pattern, measuring the disorder in liquids with high spatial and temporal resolution. The 20th century was dedicated to the development and improvement of synchrotron light sources with an ever ongoing increase of brilliance. With ultrahigh brilliance sources, the 21st century will be the century of x-ray lasers and their applications. Thus, we are already close to the dream of condensed matter and biophysics: imaging single (macro)molecules and measuring their dynamics on the femtosecond timescale to produce movies with atomic resolution.


Raman Emission By X-ray Scattering: Proceedings Of The International Conference

Raman Emission By X-ray Scattering: Proceedings Of The International Conference

Author: David L Ederer

Publisher: World Scientific

Published: 1996-09-20

Total Pages: 248

ISBN-13: 9814547255

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The Raman Emission by X-rays (REX-I) Workshop focused on Raman Scattering of x-rays mostly from Synchrotron Radiation Sources. The advent of new high brightness sources of x-ray radiation has given new impetus to this tantalizing technique that has offered ways of obtaining new insights into the atomic and electronic structure of solids and gases, but which has been limited by weak sources of excitation. In the last five years, Raman scattering by x-rays has been observed an ubiquitous phenomena. It has been applied to yield new information about the band structure of solids and about the electronic structure of atoms. It was the object of this workshop to identify and define key issues in this rapidly developing subfield of x-ray physics by gathering together a group of theorists and experimentalists, and by providing overlap between atomic and condensed matter physics. The workshop aimed to achieve this end by providing an environment to discuss the latest developments and to initiate cross fertilization in the difference areas.


Spectroscopy of Complex Oxide Interfaces

Spectroscopy of Complex Oxide Interfaces

Author: Claudia Cancellieri

Publisher: Springer

Published: 2018-04-09

Total Pages: 326

ISBN-13: 3319749897

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This book summarizes the most recent and compelling experimental results for complex oxide interfaces. The results of this book were obtained with the cutting-edge photoemission technique at highest energy resolution. Due to their fascinating properties for new-generation electronic devices and the challenge of investigating buried regions, the book chiefly focuses on complex oxide interfaces. The crucial feature of exploring buried interfaces is the use of soft X-ray angle-resolved photoemission spectroscopy (ARPES) operating on the energy range of a few hundred eV to increase the photoelectron mean free path, enabling the photons to penetrate through the top layers – in contrast to conventional ultraviolet (UV)-ARPES techniques. The results presented here, achieved by different research groups around the world, are summarized in a clearly structured way and discussed in comparison with other photoemission spectroscopy techniques and other oxide materials. They are complemented and supported by the most recent theoretical calculations as well as results of complementary experimental techniques including electron transport and inelastic resonant X-ray scattering.


Electron Dynamics by Inelastic X-Ray Scattering

Electron Dynamics by Inelastic X-Ray Scattering

Author: Winfried Schülke

Publisher: Oxford University Press, USA

Published: 2007-06-21

Total Pages: 606

ISBN-13: 0198510179

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This work offers the first comprehensive review of experimental methods, theory, and successful applications of synchrotron radiation based on inelastic X-ray scattering spectroscopy, which enables the investigation of electron dynamics in condensed matter (correlated motion and excitation).


Core Level Spectroscopy of Solids

Core Level Spectroscopy of Solids

Author: Frank de Groot

Publisher: CRC Press

Published: 2008-03-10

Total Pages: 512

ISBN-13: 1420008420

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Core level spectroscopy has become a powerful tool in the study of electronic states in solids. From fundamental aspects to the most recent developments, Core Level Spectroscopy of Solids presents the theoretical calculations, experimental data, and underlying physics of x-ray photoemission spectroscopy (XPS), x-ray absorption spectroscopy (XAS), x


Neutron and X-ray Spectroscopy

Neutron and X-ray Spectroscopy

Author: Françoise Hippert

Publisher: Springer Science & Business Media

Published: 2006-07-08

Total Pages: 580

ISBN-13: 1402033370

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- Up-to-date account of the principles and practice of inelastic and spectroscopic methods available at neutron and synchrotron sources - Multi-technique approach set around a central theme, rather than a monograph on one technique - Emphasis on the complementarity of neutron spectroscopy and X-ray spectroscopy which are usually treated in separate books