This selection of papers in the field of nonlinear optics contains reprints of original research, and general reviews written since 1960 up to the present. Brief comments by the author place each paper in a historical context of the evolution of nonlinear optics. Papers are selected from a more comprehensive bibliography either on the basis of their influence on subsequent developments or because they were originally published in journals or conference proceedings which are less easily accessible.
This textbook presents a systematic and unifying viewpoint for a wide class of nonlinear spectroscopic techniques in time domain and frequency domain. It is directed towards active researchers in physics, optics, chemistry, and materials science, as well as graduate students who enter this complex and rapidly developing field. Nonlinear optical interactions of laser fields with matter provide powerful spectroscopic tools for the understanding of microscopic interactions and dynamic processes. One of the major obstacles facing researchers in this field, however, is the flood of experimental techniques and terminologies, which create a serious language barrier. The general microscopic correlation function approach to the nonlinear optical response developed in this book is essential for understanding the relationships among different techniques and a comparison of their information content, the design of new measurements, and for a systematic comparison of the optical response of different systems such as dyes in solutions, atoms and molecules in the gas phase, liquids, molecular aggregates and superlatives, and semiconductor nanostructures. The approach is based on formulating the nonlinear response by representing the state of matter by the density matrix and following its evolution on Liouville space. Current active research areas such as femtosecond time-domain techniques, semi-classical and wave-packet dynamics, pulse shaping, pulse locking, exciton confinement, and the interplay of electronic, nuclear and field coherence are emphasized. The material has been developed from the author's highly successful interdisciplinary course at the University of Rochester attended by science and engineering graduate students.
The Handbook of Biomedical Nonlinear Optical Microscopy provides comprehensive treatment of the theories, techniques, and biomedical applications of nonlinear optics and microscopy for cell biologists, life scientists, biomedical engineers, and clinicians. The chapters are separated into basic and advanced sections, and provide both textual and graphical illustrations of all key concepts. The more basic sections are aimed at life scientists without advanced training in physics and mathematics, and tutorials are provided for the more challenging sections. The first part of the Handbook introduces the historical context of nonlinear microscopy. The second part presents the nonlinear optical theory of two- and multiphoton excited fluorescence (TPE, MPE) spectroscopy, second and third harmonic generation (SHG, THG) spectroscopy, and coherent anti-Stokes Raman spectroscopy (CARS). The third part introduces modern microscopic and spectroscopic instrumentation and techniques that are based on nonlinear optics. The fourth part provides key applications of nonlinear microscopy to the biomedical area: neurobiology, immunology, tumor biology, developmental biology, dermatology, and cellular metabolism. There are also chapters on nonlinear molecular probes, cellular damage, and nanoprocessing.
Introduction to Nonlinear Laser Spectroscopy focuses on the principles of nonlinear laser spectroscopy. This book discusses the experimental techniques of nonlinear optics and spectroscopy. Comprised of seven chapters, this book starts with an overview of the stimulated Raman effect and coherent anti-Stokes Raman spectroscopy, which can be used in a varied way to generate radiation in the ultraviolet and vacuum-ultraviolet areas. This text then explains the simplest quantum-mechanical system consisting of an isolated entity with energy eigenstates
In the last decade multiphoton excitation microscopy has emerged as an important technique with ever increasing numbers of significant applications in the fields of biology, chemistry, physics, and medicine. This volume contains key papers on the following topics: developments of nonlinear optical spectroscopy and nonlinear scanning microscopy (SHG, CARS); theory and techniques of multiphoton excitation microscopy; development of laser sources; single-molecule studies; and applications to biology, cell biology, embryology and developmental biology, neuroscience, dermatology, and optical biopsy. A comprehensive bibliography follows the reprinted papers.
TheKramers-Kronigrelationsconstitutethemathematicalformulationofthe fundamental connection between the in-phase to the out-of-phase response of a system to a sinusoidal time-varying external perturbation. Such connection exists in both classical and quantum physical systems and derives directly from the principle of causality. Apart from being of great importance in high energy physics, statistical physics, and acoustics, at present the Kramers-Kronig relations are basic and widely-accepted tools for the investigation of the linear optical properties of materials, since they allow performing the so-called inversion of optical data, i.e. acquiring knowledge on dispersive phenomena by measurements of absorptive phenomena over the whole energy spectrum or vice versa. Since the late ’80s, a growing body of theoretical results as well as of experimental evidences has shown that the Kramers-Kronig relations can be adopted for e?ciently acquiring knowledge on nonlinear optical phenomena. These results suggest that the Kramers-Kronig relations may become in a near future standard techniques in the context of nonlinear spectroscopy. Thisbookisthe?rstcomprehensivetreatisedevotedtoprovidingauni- ing picture of the physical backgrounds, of the rigorous mathematical theory, and of the applications of the Kramers-Kronig relations in both ?elds of l- ear and nonlinear optical spectroscopy. Some basic programs written for the 1 MATLAB environment are also included. This book is organized as an argumentative discourse, progressing from the linear to the nonlinear phenomena, from the general to the speci?c s- tems, and from the theoretical to the experimental results.
This book provides an up-to-date account of current trends in nonlinear optics. It is intended for researchers already engaged in the field of nonlinear optics. It may also be used by graduate students due to its comprehensive coverage and pedagogical presentation.
This selection of papers in the field of nonlinear optics contains reprints of original research, and general reviews written since 1960 up to the present. Brief comments by the author place each paper in a historical context of the evolution of nonlinear optics. Papers are selected from a more comprehensive bibliography either on the basis of their influence on subsequent developments or because they were originally published in journals or conference proceedings which are less easily accessible.
