Rate Theory Modeling and Simulation of Silicide Fuel at LWR Conditions

Rate Theory Modeling and Simulation of Silicide Fuel at LWR Conditions

Author:

Publisher:

Published: 2016

Total Pages: 33

ISBN-13:

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As a promising candidate for the accident tolerant fuel (ATF) used in light water reactors (LWRs), the fuel performance of uranium silicide (U3Si2) at LWR conditions need to be well-understood. In this report, rate theory model was developed based on existing experimental data and density functional theory (DFT) calculations so as to predict the fission gas behavior in U3Si2 at LWR conditions. The fission gas behavior of U3Si2 can be divided into three temperature regimes. During steady-state operation, the majority of the fission gas stays in intragranular bubbles, whereas the dominance of intergranular bubbles and fission gas release only occurs beyond 1000 K. The steady-state rate theory model was also used as reference to establish a gaseous swelling correlation of U3Si2 for the BISON code. Meanwhile, the overpressurized bubble model was also developed so that the fission gas behavior at LOCA can be simulated. LOCA simulation showed that intragranular bubbles are still dominant after a 70 second LOCA, resulting in a controllable gaseous swelling. The fission gas behavior of U3Si2 at LWR conditions is benign according to the rate theory prediction at both steady-state and LOCA conditions, which provides important references to the qualification of U3Si2 as a LWR fuel material with excellent fuel performance and enhanced accident tolerance.


Rate Theory Modeling an Simulations of Silicide Fuel at LWR Conditions

Rate Theory Modeling an Simulations of Silicide Fuel at LWR Conditions

Author:

Publisher:

Published: 2015

Total Pages: 30

ISBN-13:

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Uranium silicide (U3Si2) fuel has higher thermal conductivity and higher uranium density, making it a promising candidate for the accident-tolerant fuel (ATF) used in light water reactors (LWRs). However, previous studies on the fuel performance of U3Si2, including both experimental and computational approaches, have been focusing on the irradiation conditions in research reactors, which usually involve low operation temperatures and high fuel burnups. Thus, it is important to examine the fuel performance of U3Si2 at typical LWR conditions so as to evaluate the feasibility of replacing conventional uranium dioxide fuel with this silicide fuel material. As in-reactor irradiation experiments involve significant time and financial cost, it is appropriate to utilize modeling tools to estimate the behavior of U3Si2 in LWRs based on all those available research reactor experimental references and state-of-the-art density functional theory (DFT) calculation capabilities at the early development stage. Hence, in this report, a comprehensive investigation of the fission gas swelling behavior of U3Si2 at LWR conditions is introduced. The modeling efforts mentioned in this report was based on the rate theory (RT) model of fission gas bubble evolution that has been successfully applied for a variety of fuel materials at devious reactor conditions. Both existing experimental data and DFT-calculated results were used for the optimization of the parameters adopted by the RT model. Meanwhile, the fuel-cladding interaction was captured by the coupling of the RT model with simplified mechanical correlations. Therefore, the swelling behavior of U3Si2 fuel and its consequent interaction with cladding in LWRs was predicted by the rate theory modeling, providing valuable information for the development of U3Si2 fuel as an accident-tolerant alternative for uranium dioxide.


Multi-Physics and Multi-Scale Modeling and Simulation Methods for Nuclear Reactor Application

Multi-Physics and Multi-Scale Modeling and Simulation Methods for Nuclear Reactor Application

Author: Xingjie Peng

Publisher: Frontiers Media SA

Published: 2024-02-28

Total Pages: 105

ISBN-13: 2832545378

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A nuclear reactor operates in an environment where complex multi-physics and multi-scale phenomena exist, and it requires consideration of coupling among neutronics, thermal hydraulics, fuel performance, chemical dynamics, and coupling between the reactor core and first circuit. Safe, reliable, and economical operation can be achieved by leveraging high-fidelity numerical simulation, and proper considerations for coupling among different physics and required to provide powerful numerical simulation tools. In the past simplistic models for some of the physics phenomena are used, with the recent development of advanced numerical methods, software design, and high-performance computing power, the appeal of multi-physics and multi-scale modeling and simulation has been broadened.


Safety of Light Water Reactor Fuel with Silicon Carbide Cladding

Safety of Light Water Reactor Fuel with Silicon Carbide Cladding

Author: Youho Lee

Publisher:

Published: 2013

Total Pages: 319

ISBN-13:

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Structural aspects of the performance of light water reactor (LWR) fuel rod with triplex silicon carbide (SiC) cladding - an emerging option to replace the zirconium alloy cladding - are assessed. Its behavior under accident conditions is examined with an integrated approach of experiments, modeling, and simulation. High temperature (1100°C~1500°C) steam oxidation experiments demonstrated that the oxidation of monolithic SiC is about three orders of magnitude slower than that of zirconium alloys, and with a weaker impact on mechanical strength. This, along with the presence of the environmental barrier coating around the load carrying intermediate layer of SiC fiber composite, diminishes the importance of oxidation for cladding failure mechanisms. Thermal shock experiments showed strength retention for both [alpha]-SiC and [beta]-SiC, as well as A12O3 samples quenched from temperatures up to 1260°C in saturated water. The initial heat transfer upon the solid - fluid contact in the quenching transient is found to be a controlling factor in the potential for brittle fracture. This implies that SiC would not fail by thermal shock induced fracture during the reflood phase of a loss of coolant accident, which includes fuel-cladding quenching by emergency coolant at saturation conditions. A thermo-mechanical model for stress distribution and Weibull statistical fracture of laminated SiC cladding during normal and accident conditions is developed. It is coupled to fuel rod performance code FRAPCON-3.4 (modified here for SiC) and RELAP-5 (to determine coolant conditions). It is concluded that a PWR fuel rod with SiC cladding can extend the fuel residence time in the core, while keeping the internal pressure level within the safety assurance limit during steady-state and loss of coolant accidents. Peak burnup of 93 MWD/kgU (10% central void in fuel pellets) at 74 months of in-core residence time is found achievable with conventional PWR fuel rod design, but with an extended plenum length (70 cm). An easier to manufacture, 30% larger SiC cladding thickness requires an improved thermal conductivity of the composite layer to reduce thermal stress levels under steady-state operation to avoid failure at the same burnup. A larger Weibull modulus of the SiC cladding improves chances of avoiding brittle failure.


Comprehensive Nuclear Materials

Comprehensive Nuclear Materials

Author:

Publisher: Elsevier

Published: 2020-07-22

Total Pages: 4871

ISBN-13: 0081028660

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Materials in a nuclear environment are exposed to extreme conditions of radiation, temperature and/or corrosion, and in many cases the combination of these makes the material behavior very different from conventional materials. This is evident for the four major technological challenges the nuclear technology domain is facing currently: (i) long-term operation of existing Generation II nuclear power plants, (ii) the design of the next generation reactors (Generation IV), (iii) the construction of the ITER fusion reactor in Cadarache (France), (iv) and the intermediate and final disposal of nuclear waste. In order to address these challenges, engineers and designers need to know the properties of a wide variety of materials under these conditions and to understand the underlying processes affecting changes in their behavior, in order to assess their performance and to determine the limits of operation. Comprehensive Nuclear Materials, Second Edition, Seven Volume Set provides broad ranging, validated summaries of all the major topics in the field of nuclear material research for fission as well as fusion reactor systems. Attention is given to the fundamental scientific aspects of nuclear materials: fuel and structural materials for fission reactors, waste materials, and materials for fusion reactors. The articles are written at a level that allows undergraduate students to understand the material, while providing active researchers with a ready reference resource of information. Most of the chapters from the first Edition have been revised and updated and a significant number of new topics are covered in completely new material. During the ten years between the two editions, the challenge for applications of nuclear materials has been significantly impacted by world events, public awareness, and technological innovation. Materials play a key role as enablers of new technologies, and we trust that this new edition of Comprehensive Nuclear Materials has captured the key recent developments. Critically reviews the major classes and functions of materials, supporting the selection, assessment, validation and engineering of materials in extreme nuclear environments Comprehensive resource for up-to-date and authoritative information which is not always available elsewhere, even in journals Provides an in-depth treatment of materials modeling and simulation, with a specific focus on nuclear issues Serves as an excellent entry point for students and researchers new to the field


Fundamentals of Electromigration-Aware Integrated Circuit Design

Fundamentals of Electromigration-Aware Integrated Circuit Design

Author: Jens Lienig

Publisher: Springer

Published: 2018-02-23

Total Pages: 171

ISBN-13: 3319735586

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The book provides a comprehensive overview of electromigration and its effects on the reliability of electronic circuits. It introduces the physical process of electromigration, which gives the reader the requisite understanding and knowledge for adopting appropriate counter measures. A comprehensive set of options is presented for modifying the present IC design methodology to prevent electromigration. Finally, the authors show how specific effects can be exploited in present and future technologies to reduce electromigration’s negative impact on circuit reliability.


Strategy and Methodology for Radioactive Waste Characterization

Strategy and Methodology for Radioactive Waste Characterization

Author: International Atomic Energy Agency

Publisher: IAEA

Published: 2007

Total Pages: 188

ISBN-13:

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Over the past decade significant progress has been achieved in the development of waste characterization and control procedures and equipment as a direct response to ever-increasing requirements for quality and reliability of information on waste characteristics. Failure in control procedures at any step can have important, adverse consequences and may result in producing waste packages which are not compliant with the waste acceptance criteria for disposal, thereby adversely impacting the repository. The information and guidance included in this publication corresponds to recent achievements and reflects the optimum approaches, thereby reducing the potential for error and enhancing the quality of the end product. -- Publisher's description.